Extraordinary activity of nanodispersed bimetallic nife phosphide catalysts for the conversion of a biomass model compound

S. Ted Oyama, Ara Cho, Jieun Shin, Atsushi Takagaki, Ryuji Kikuchi

研究成果: 書籍/レポート タイプへの寄稿会議への寄与

抄録

The present work deals with the development of new catalysts, transition metal phosphides, which have outstanding activity for hydrodeoxygenation of pyrolysis oil. The study is significant as it leads to the production of high-energy content liquid fuels. Pyrolysis of biomass is a thermal conversion process that produces liquid fuels and chemicals, and is a promising technology to compete with and eventually replace non-renewable fossil fuels. The model substrate 2-methyltetrahydrofuran is studied by kinetic and spectroscopic methods to uncover the important steps involved in the reaction. On the most active catalyst, Ni2P, the studies indicate that the rate-determining step involves a single Ni atom. In situ infrared measurements are used to identify adsorbed reactive intermediates during reaction and give support for the reaction mechanism. The studies are important because they allow understanding of reactivity at a nanoscale level and lead to the design of more active catalysts.

本文言語英語
ホスト出版物のタイトルTechnical Proceedings of the 2013 NSTI Nanotechnology Conference and Expo, NSTI-Nanotech 2013
ページ444-447
ページ数4
出版ステータス出版済み - 2013
外部発表はい
イベントNanotechnology 2013: Advanced Materials, CNTs, Particles, Films and Composites - 2013 NSTI Nanotechnology Conference and Expo, NSTI-Nanotech 2013 - Washington, DC, 米国
継続期間: 5月 12 20135月 16 2013

出版物シリーズ

名前Technical Proceedings of the 2013 NSTI Nanotechnology Conference and Expo, NSTI-Nanotech 2013
1

その他

その他Nanotechnology 2013: Advanced Materials, CNTs, Particles, Films and Composites - 2013 NSTI Nanotechnology Conference and Expo, NSTI-Nanotech 2013
国/地域米国
CityWashington, DC
Period5/12/135/16/13

!!!All Science Journal Classification (ASJC) codes

  • バイオテクノロジー

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