TY - JOUR
T1 - Energy-Saving CO2Capture by H2Gas Stripping for Integrating CO2Separation and Conversion Processes
AU - Machida, Hiroshi
AU - Esaki, Takehiro
AU - Esaki, Takehiro
AU - Yamaguchi, Tsuyoshi
AU - Norinaga, Koyo
N1 - Publisher Copyright:
Copyright © 2020 American Chemical Society.
PY - 2020/6/15
Y1 - 2020/6/15
N2 - CO2 capture and utilization technology, such as converting CO2 to fuel or chemicals by renewable energy-derived H2, has been promoted for recent decades. Herein, a process is proposed that saves considerable amounts of energy by integrating the CO2 separation and conversion processes. In the case of the method of amine absorption, supplying H2 to the bottom of the desorber reduces the regeneration temperature, which can reduce the process exergy. If combined with reaction heat recovery using a heat pump system, a considerable amount of energy can be saved. The recovered mixture of CO2 and H2 gas is then used directly as a raw reaction material. Herein, the proposed stripping regeneration process is compared on theoretical and equilibrium bases, with the conventional monoethanolamine method and the phase-separation solvent method developed by the authors. Using the phase-separation solvent leads to lower energy in the stripping regeneration.
AB - CO2 capture and utilization technology, such as converting CO2 to fuel or chemicals by renewable energy-derived H2, has been promoted for recent decades. Herein, a process is proposed that saves considerable amounts of energy by integrating the CO2 separation and conversion processes. In the case of the method of amine absorption, supplying H2 to the bottom of the desorber reduces the regeneration temperature, which can reduce the process exergy. If combined with reaction heat recovery using a heat pump system, a considerable amount of energy can be saved. The recovered mixture of CO2 and H2 gas is then used directly as a raw reaction material. Herein, the proposed stripping regeneration process is compared on theoretical and equilibrium bases, with the conventional monoethanolamine method and the phase-separation solvent method developed by the authors. Using the phase-separation solvent leads to lower energy in the stripping regeneration.
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U2 - 10.1021/acssuschemeng.0c02459
DO - 10.1021/acssuschemeng.0c02459
M3 - Article
AN - SCOPUS:85086565180
SN - 2168-0485
VL - 8
SP - 8732
EP - 8740
JO - ACS Sustainable Chemistry and Engineering
JF - ACS Sustainable Chemistry and Engineering
IS - 23
ER -