Comparison of humidified hydrogen and partly pre-reformed natural gas as fuel for solid oxide fuel cells applying computational fluid dynamics

Martin Andersson, Hironori Nakajima, Tatsumi Kitahara, Akira Shimizu, Takahiro Koshiyama, Hedvig Paradis, Jinliang Yuan, Bengt Sundén

研究成果: ジャーナルへの寄稿学術誌査読

48 被引用数 (Scopus)

抄録

A three-dimensional computational fluid dynamics (CFD) approach based on the finite element method (FEM) is used to investigate a solid oxide fuel cell (SOFC). Governing equations for heat, gas-phase species, electron, ion and momentum transport are implemented and coupled to kinetics describing electrochemical as well as internal reforming reactions. The model cell design is based on a cell from Ningbo Institute of Material Technology and Engineering in China and the electrochemical area-to-volume ratios are based on experimental work performed at Kyushu University in Japan. A parameter study is performed focusing on the inlet fuel composition, where humidified hydrogen, 30% pre-reformed natural gas (as defined by IEA) and 50% pre-reformed natural gas (as defined by Kyushu University) are compared. It is found that when 30% pre-reformed natural gas is supplied as fuel the air mass flow rate is halved, compared to the case with humidified hydrogen, keeping the inlet and outlet temperatures constant. The current density is decreased but the fuel utilization is kept at 80%. It is found that the cathode support layer has a significant oxygen gas-phase resistance in the direction normal to the cathode/electrolyte interface (at positions under the interconnect ribs), as well as an electron resistance inside the cathode (at positions under the air channel) in the same direction. The methane steam reforming reaction is shown, both according to the experiments and to the models, to proceed along the main flow direction throughout the cell.

本文言語英語
ページ(範囲)1008-1022
ページ数15
ジャーナルInternational Journal of Heat and Mass Transfer
77
DOI
出版ステータス出版済み - 10月 2014

!!!All Science Journal Classification (ASJC) codes

  • 凝縮系物理学
  • 機械工学
  • 流体および伝熱

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