TY - JOUR
T1 - A new strategy for membrane-based direct air capture
AU - Fujikawa, Shigenori
AU - Selyanchyn, Roman
AU - Kunitake, Toyoki
N1 - Funding Information:
Acknowledgements This work was supported by the World Premier International Research Center Initiative (WPI), sponsored by the Japanese Ministry of Education, Culture, Sports, Science, and Technology. SF acknowledges the Japan Society for Promotion of Science (JSPS) for a Grant-in-Aid for Scientific Research (B) (20H02781). RS acknowledges the Japan Society for Promotion of Science (JSPS) for a Grant-in-Aid for Early Career Scientists (19K15342).
PY - 2020/10/15
Y1 - 2020/10/15
N2 - Direct CO2 capture from the air, so-called direct air capture (DAC), has become inevitable to reduce the concentration of CO2 in the atmosphere. Current DAC technologies consider only sorbent-based systems. Recently, there have been reports that show ultrahigh CO2 permeances in gas separation membranes and thus membrane separation could be a potential new technology for DAC in addition to sorbent-based CO2 capture. The simulation of chemical processes has been well established and is commonly used for the development and performance assessment of industrial chemical processes. These simulations offer a credible assessment of the feasibility of membrane-based DAC (m-DAC). In this paper, we discuss the potential of m-DAC considering the state-of-the-art performance of organic polymer membranes. The multistage membrane separation process was employed in process simulation to estimate the energy requirements for m-DAC. Based on the analysis, we propose the target membrane separation performance required for m-DAC with competitive energy expenses. Finally, we discuss the direction of future membrane development for DAC.
AB - Direct CO2 capture from the air, so-called direct air capture (DAC), has become inevitable to reduce the concentration of CO2 in the atmosphere. Current DAC technologies consider only sorbent-based systems. Recently, there have been reports that show ultrahigh CO2 permeances in gas separation membranes and thus membrane separation could be a potential new technology for DAC in addition to sorbent-based CO2 capture. The simulation of chemical processes has been well established and is commonly used for the development and performance assessment of industrial chemical processes. These simulations offer a credible assessment of the feasibility of membrane-based DAC (m-DAC). In this paper, we discuss the potential of m-DAC considering the state-of-the-art performance of organic polymer membranes. The multistage membrane separation process was employed in process simulation to estimate the energy requirements for m-DAC. Based on the analysis, we propose the target membrane separation performance required for m-DAC with competitive energy expenses. Finally, we discuss the direction of future membrane development for DAC.
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U2 - 10.1038/s41428-020-00429-z
DO - 10.1038/s41428-020-00429-z
M3 - Review article
AN - SCOPUS:85092671966
SN - 0032-3896
VL - 53
SP - 111
EP - 119
JO - Polymer Journal
JF - Polymer Journal
IS - 1
ER -