Spallation reaction study for the long-lived fission products in nuclear waste: Cross section measurements for 137Cs, 90Sr and 107Pd using inverse kinematics method

He Wang; Hideaki Otsu; Hiroyoshi Sakurai; Deuksoon Ahn; Nobuyuki Chiga; Pieter Doornenbal; Naoki Fukuda; Tadaaki Isobe; Toshiyuki Kubo; Shigeru Kubono; Giusseppe Lorusso; Pär Anders Söderström; Hiroshi Suzuki; Hiroyuki Takeda; Yasushi Watanabe; Koichi Yoshida; Teiichiro Matsuzaki; Yohei Shimizu; Toshiyuki Sumikama; Meiko Uesaka; Shoichiro Kawase; Keita Nakano; Yukinobu Watanabe; Shouhei Araki; Tadahiro Kin; Satoshi Takeuchi; Yasuhiro Togano; Takashi Nakamura; Yosuke Kondo; Tomoyuki Ozaki; Atsumi Saito; Junichi Tsubota; Masayuki Aikawa; Ayano Makinaga; Takashi Ando; Shunpei Koyama; Satoru Momiyama; Shunsuke Nagamine; Megumi Niikura; Takeshi Saito; Ryo Taniuchi; Kathrin Wimmer; Shunsuke Kawakami; Yukie Maeda; Tatsuya Yamamoto; Yoshiaki Shiga; Masafumi Matsushita; Shin'Ichiro Michimasa; Susumu Shimoura

doi:10.1016/j.egypro.2017.09.434

Spallation reaction study for the long-lived fission products in nuclear waste: Cross section measurements for ¹³⁷Cs, ⁹⁰Sr and ¹⁰⁷Pd using inverse kinematics method

He Wang, Hideaki Otsu, Hiroyoshi Sakurai, Deuksoon Ahn, Nobuyuki Chiga, Pieter Doornenbal, Naoki Fukuda, Tadaaki Isobe, Toshiyuki Kubo, Shigeru Kubono, Giusseppe Lorusso, Pär Anders Söderström, Hiroshi Suzuki, Hiroyuki Takeda, Yasushi Watanabe, Koichi Yoshida, Teiichiro Matsuzaki, Yohei Shimizu, Toshiyuki Sumikama, Meiko UesakaShoichiro Kawase, Keita Nakano, Yukinobu Watanabe, Shouhei Araki, Tadahiro Kin, Satoshi Takeuchi, Yasuhiro Togano, Takashi Nakamura, Yosuke Kondo, Tomoyuki Ozaki, Atsumi Saito, Junichi Tsubota, Masayuki Aikawa, Ayano Makinaga, Takashi Ando, Shunpei Koyama, Satoru Momiyama, Shunsuke Nagamine, Megumi Niikura, Takeshi Saito, Ryo Taniuchi, Kathrin Wimmer, Shunsuke Kawakami, Yukie Maeda, Tatsuya Yamamoto, Yoshiaki Shiga, Masafumi Matsushita, Shin'Ichiro Michimasa, Susumu Shimoura

Engineering Science for Advanced energy system

Research output: Contribution to journal › Conference article › peer-review

4 Citations (Scopus)

Abstract

Spallation reaction study has been performed for the long-lived fission products ¹³⁷Cs, ⁹⁰Sr and ¹⁰⁷Pd. Isotopic cross sections on proton and deuteron were obtained by using the inverse kinematics technique at the RIKEN Radioactive Isotope Beam Factory. It was found that the deuteron-induced cross sections are larger than the proton-induced ones for the light-mass products. The experimental data were compared with the SPACS semi-empirical parameterization and a theoretical calculation including both the intra-nuclear cascade and evaporation models by the PHITS transport code. It was found that the spallation reaction could be a promising mechanism for the transmutation of ¹³⁷Cs and ⁹⁰Sr due to the large total cross section.

Original language	English
Pages (from-to)	127-132
Number of pages	6
Journal	Energy Procedia
Volume	131
DOIs	https://doi.org/10.1016/j.egypro.2017.09.434
Publication status	Published - 2017
Event	5th International Symposium on Innovative Nuclear Energy Systems, INES-5 2016 - Tokyo, Japan Duration: Oct 31 2017 → Nov 2 2017

All Science Journal Classification (ASJC) codes

Energy(all)

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10.1016/j.egypro.2017.09.434

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Wang, H., Otsu, H., Sakurai, H., Ahn, D., Chiga, N., Doornenbal, P., Fukuda, N., Isobe, T., Kubo, T., Kubono, S., Lorusso, G., Söderström, P. A., Suzuki, H., Takeda, H., Watanabe, Y., Yoshida, K., Matsuzaki, T., Shimizu, Y., Sumikama, T., ... Shimoura, S. (2017). Spallation reaction study for the long-lived fission products in nuclear waste: Cross section measurements for ¹³⁷Cs, ⁹⁰Sr and ¹⁰⁷Pd using inverse kinematics method. Energy Procedia, 131, 127-132. https://doi.org/10.1016/j.egypro.2017.09.434

Wang, H, Otsu, H, Sakurai, H, Ahn, D, Chiga, N, Doornenbal, P, Fukuda, N, Isobe, T, Kubo, T, Kubono, S, Lorusso, G, Söderström, PA, Suzuki, H, Takeda, H, Watanabe, Y, Yoshida, K, Matsuzaki, T, Shimizu, Y, Sumikama, T, Uesaka, M, Kawase, S, Nakano, K, Watanabe, Y, Araki, S, Kin, T, Takeuchi, S, Togano, Y, Nakamura, T, Kondo, Y, Ozaki, T, Saito, A, Tsubota, J, Aikawa, M, Makinaga, A, Ando, T, Koyama, S, Momiyama, S, Nagamine, S, Niikura, M, Saito, T, Taniuchi, R, Wimmer, K, Kawakami, S, Maeda, Y, Yamamoto, T, Shiga, Y, Matsushita, M, Michimasa, SI & Shimoura, S 2017, 'Spallation reaction study for the long-lived fission products in nuclear waste: Cross section measurements for ¹³⁷Cs, ⁹⁰Sr and ¹⁰⁷Pd using inverse kinematics method', Energy Procedia, vol. 131, pp. 127-132. https://doi.org/10.1016/j.egypro.2017.09.434

@article{044a1e4ddf04457daccb398d5debcdac,

title = "Spallation reaction study for the long-lived fission products in nuclear waste: Cross section measurements for 137Cs, 90Sr and 107Pd using inverse kinematics method",

abstract = "Spallation reaction study has been performed for the long-lived fission products 137Cs, 90Sr and 107Pd. Isotopic cross sections on proton and deuteron were obtained by using the inverse kinematics technique at the RIKEN Radioactive Isotope Beam Factory. It was found that the deuteron-induced cross sections are larger than the proton-induced ones for the light-mass products. The experimental data were compared with the SPACS semi-empirical parameterization and a theoretical calculation including both the intra-nuclear cascade and evaporation models by the PHITS transport code. It was found that the spallation reaction could be a promising mechanism for the transmutation of 137Cs and 90Sr due to the large total cross section.",

author = "He Wang and Hideaki Otsu and Hiroyoshi Sakurai and Deuksoon Ahn and Nobuyuki Chiga and Pieter Doornenbal and Naoki Fukuda and Tadaaki Isobe and Toshiyuki Kubo and Shigeru Kubono and Giusseppe Lorusso and S{\"o}derstr{\"o}m, {P{\"a}r Anders} and Hiroshi Suzuki and Hiroyuki Takeda and Yasushi Watanabe and Koichi Yoshida and Teiichiro Matsuzaki and Yohei Shimizu and Toshiyuki Sumikama and Meiko Uesaka and Shoichiro Kawase and Keita Nakano and Yukinobu Watanabe and Shouhei Araki and Tadahiro Kin and Satoshi Takeuchi and Yasuhiro Togano and Takashi Nakamura and Yosuke Kondo and Tomoyuki Ozaki and Atsumi Saito and Junichi Tsubota and Masayuki Aikawa and Ayano Makinaga and Takashi Ando and Shunpei Koyama and Satoru Momiyama and Shunsuke Nagamine and Megumi Niikura and Takeshi Saito and Ryo Taniuchi and Kathrin Wimmer and Shunsuke Kawakami and Yukie Maeda and Tatsuya Yamamoto and Yoshiaki Shiga and Masafumi Matsushita and Shin'Ichiro Michimasa and Susumu Shimoura",

note = "Funding Information: The authors thank the accelerator staff of RIKEN Nishina Center for providing the U beam. Part of this work was supported by ImPACT program of Council for Science, Technology and Innovation (Cabinet Office, Government of Japan). Publisher Copyright: {\textcopyright} 2017 The Authors. Published by Elsevier Ltd.; 5th International Symposium on Innovative Nuclear Energy Systems, INES-5 2016 ; Conference date: 31-10-2017 Through 02-11-2017",

year = "2017",

doi = "10.1016/j.egypro.2017.09.434",

language = "English",

volume = "131",

pages = "127--132",

journal = "Energy Procedia",

issn = "1876-6102",

publisher = "Elsevier BV",

}

TY - JOUR

T1 - Spallation reaction study for the long-lived fission products in nuclear waste

T2 - 5th International Symposium on Innovative Nuclear Energy Systems, INES-5 2016

AU - Wang, He

AU - Otsu, Hideaki

AU - Sakurai, Hiroyoshi

AU - Ahn, Deuksoon

AU - Chiga, Nobuyuki

AU - Doornenbal, Pieter

AU - Fukuda, Naoki

AU - Isobe, Tadaaki

AU - Kubo, Toshiyuki

AU - Kubono, Shigeru

AU - Lorusso, Giusseppe

AU - Söderström, Pär Anders

AU - Suzuki, Hiroshi

AU - Takeda, Hiroyuki

AU - Watanabe, Yasushi

AU - Yoshida, Koichi

AU - Matsuzaki, Teiichiro

AU - Shimizu, Yohei

AU - Sumikama, Toshiyuki

AU - Uesaka, Meiko

AU - Kawase, Shoichiro

AU - Nakano, Keita

AU - Watanabe, Yukinobu

AU - Araki, Shouhei

AU - Kin, Tadahiro

AU - Takeuchi, Satoshi

AU - Togano, Yasuhiro

AU - Nakamura, Takashi

AU - Kondo, Yosuke

AU - Ozaki, Tomoyuki

AU - Saito, Atsumi

AU - Tsubota, Junichi

AU - Aikawa, Masayuki

AU - Makinaga, Ayano

AU - Ando, Takashi

AU - Koyama, Shunpei

AU - Momiyama, Satoru

AU - Nagamine, Shunsuke

AU - Niikura, Megumi

AU - Saito, Takeshi

AU - Taniuchi, Ryo

AU - Wimmer, Kathrin

AU - Kawakami, Shunsuke

AU - Maeda, Yukie

AU - Yamamoto, Tatsuya

AU - Shiga, Yoshiaki

AU - Matsushita, Masafumi

AU - Michimasa, Shin'Ichiro

AU - Shimoura, Susumu

N1 - Funding Information: The authors thank the accelerator staff of RIKEN Nishina Center for providing the U beam. Part of this work was supported by ImPACT program of Council for Science, Technology and Innovation (Cabinet Office, Government of Japan). Publisher Copyright: © 2017 The Authors. Published by Elsevier Ltd.

PY - 2017

Y1 - 2017

N2 - Spallation reaction study has been performed for the long-lived fission products 137Cs, 90Sr and 107Pd. Isotopic cross sections on proton and deuteron were obtained by using the inverse kinematics technique at the RIKEN Radioactive Isotope Beam Factory. It was found that the deuteron-induced cross sections are larger than the proton-induced ones for the light-mass products. The experimental data were compared with the SPACS semi-empirical parameterization and a theoretical calculation including both the intra-nuclear cascade and evaporation models by the PHITS transport code. It was found that the spallation reaction could be a promising mechanism for the transmutation of 137Cs and 90Sr due to the large total cross section.

AB - Spallation reaction study has been performed for the long-lived fission products 137Cs, 90Sr and 107Pd. Isotopic cross sections on proton and deuteron were obtained by using the inverse kinematics technique at the RIKEN Radioactive Isotope Beam Factory. It was found that the deuteron-induced cross sections are larger than the proton-induced ones for the light-mass products. The experimental data were compared with the SPACS semi-empirical parameterization and a theoretical calculation including both the intra-nuclear cascade and evaporation models by the PHITS transport code. It was found that the spallation reaction could be a promising mechanism for the transmutation of 137Cs and 90Sr due to the large total cross section.

UR - http://www.scopus.com/inward/record.url?scp=85041997627&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=85041997627&partnerID=8YFLogxK

U2 - 10.1016/j.egypro.2017.09.434

DO - 10.1016/j.egypro.2017.09.434

M3 - Conference article

AN - SCOPUS:85041997627

SN - 1876-6102

VL - 131

SP - 127

EP - 132

JO - Energy Procedia

JF - Energy Procedia

Y2 - 31 October 2017 through 2 November 2017

ER -

Spallation reaction study for the long-lived fission products in nuclear waste: Cross section measurements for ¹³⁷Cs, ⁹⁰Sr and ¹⁰⁷Pd using inverse kinematics method

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