TY - JOUR
T1 - High-efficiency light emission by means of exciton–surface-plasmon coupling
AU - Okamoto, Koichi
AU - Funato, Mitsuru
AU - Kawakami, Yoichi
AU - Tamada, Kaoru
N1 - Funding Information:
This work was supported by Grants-in-Aid for Scientific Research of types B (26289109) and S (15H05732). This work was also partially supported by the Precursory Research for Embryonic Science and Technology (PRESTO) program of the Japan Science and Technology Agency (JST) and the Cooperative Research Program of the “Network Joint Research Center for Materials and Devices”.
Publisher Copyright:
© 2017 Elsevier B.V.
PY - 2017/9
Y1 - 2017/9
N2 - Coupling between surface plasmons (SPs) and excitons can be used to enhance the emission efficiencies of light-emitting materials and devices. This approach had been theoretically predicted and, in 2004, was experimentally demonstrated by our group for enhancing the visible emission from InGaN/GaN quantum wells (QWs). Exciton–SP coupling increases the spontaneous emission rates of the excited states, causes a relative reduction in nonradiative relaxation, and ultimately increases the internal quantum efficiencies (IQEs) of such devices. Here, we present a brief history of the increases in emission efficiency that have been achieved and the underlying mechanism thereof. This method has the potential to enable the development of high-efficiency light-emitting diodes (LEDs), eventually leading to the replacement of fluorescent lights with solid-state light sources. After the initial discovery of this phenomenon, many device structures were proposed and reported; however, their emission efficiencies have thus far remained insufficient for practical application. Here, we also present recent progress on device applications and the current problems that must be solved. Finally, we explain the future possibilities regarding the extension of SP-enhanced light emission over a broader wavelength region, from the deep ultraviolet (UV) to the infrared (IR).
AB - Coupling between surface plasmons (SPs) and excitons can be used to enhance the emission efficiencies of light-emitting materials and devices. This approach had been theoretically predicted and, in 2004, was experimentally demonstrated by our group for enhancing the visible emission from InGaN/GaN quantum wells (QWs). Exciton–SP coupling increases the spontaneous emission rates of the excited states, causes a relative reduction in nonradiative relaxation, and ultimately increases the internal quantum efficiencies (IQEs) of such devices. Here, we present a brief history of the increases in emission efficiency that have been achieved and the underlying mechanism thereof. This method has the potential to enable the development of high-efficiency light-emitting diodes (LEDs), eventually leading to the replacement of fluorescent lights with solid-state light sources. After the initial discovery of this phenomenon, many device structures were proposed and reported; however, their emission efficiencies have thus far remained insufficient for practical application. Here, we also present recent progress on device applications and the current problems that must be solved. Finally, we explain the future possibilities regarding the extension of SP-enhanced light emission over a broader wavelength region, from the deep ultraviolet (UV) to the infrared (IR).
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U2 - 10.1016/j.jphotochemrev.2017.05.005
DO - 10.1016/j.jphotochemrev.2017.05.005
M3 - Review article
AN - SCOPUS:85020699870
SN - 1389-5567
VL - 32
SP - 58
EP - 77
JO - Journal of Photochemistry and Photobiology C: Photochemistry Reviews
JF - Journal of Photochemistry and Photobiology C: Photochemistry Reviews
ER -